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Atomically Layered and Ordered Rare-Earth i-MAX Phases: A New Class of Magnetic Quaternary Compounds
Linkoping Univ, Thin Film Phys Div, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden.
Linkoping Univ, Thin Film Phys Div, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden.
Linkoping Univ, Thin Film Phys Div, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden.
Linkoping Univ, Thin Film Phys Div, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden;Oak Ridge Natl Lab, Neutron Scattering Div, Oak Ridge, TN 37831 USA.
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2019 (engelsk)Inngår i: Chemistry of Materials, ISSN 0897-4756, E-ISSN 1520-5002, Vol. 31, nr 7, s. 2476-2485Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

In 2017, we discovered quaternary i-MAX phases atomically layered solids, where M is an early transition metal, A is an A group element, and X is C—with a (M12/3M21/3)2AC chemistry, where the M1 and M2 atoms are in-plane ordered. Herein, we report the discovery of a class of magnetic i-MAX phases in which bilayers of a quasi-2D magnetic frustrated triangular lattice overlay a Mo honeycomb arrangement and an Al Kagome lattice. The chemistry of this family is (Mo2/3RE1/3)2AlC, and the rare-earth, RE, elements are Ce, Pr, Nd, Sm, Gd, Tb, Dy, Ho, Er, Tm, and Lu. The magnetic properties were characterized and found to display a plethora of ground states, resulting from an interplay of competing magnetic interactions in the presence of magnetocrystalline anisotropy.

sted, utgiver, år, opplag, sider
2019. Vol. 31, nr 7, s. 2476-2485
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URN: urn:nbn:se:uu:diva-382860DOI: 10.1021/acs.chemmater.8b05298ISI: 000464477100029OAI: oai:DiVA.org:uu-382860DiVA, id: diva2:1315090
Forskningsfinansiär
Knut and Alice Wallenberg Foundation, KAW 2015.0043Swedish Research Council, 642-2013-8020Swedish Research Council, 2015-00607Swedish Research Council, 621-2014-4890Swedish National Infrastructure for Computing (SNIC)German Research Foundation (DFG), SA 3095/2-1Tilgjengelig fra: 2019-05-10 Laget: 2019-05-10 Sist oppdatert: 2019-05-10bibliografisk kontrollert

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