uu.seUppsala universitets publikationer
Ändra sökning
RefereraExporteraLänk till posten
Permanent länk

Direktlänk
Referera
Referensformat
  • apa
  • ieee
  • modern-language-association
  • vancouver
  • Annat format
Fler format
Språk
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Annat språk
Fler språk
Utmatningsformat
  • html
  • text
  • asciidoc
  • rtf
Fabrication of ultra-pure gold nanoparticles capped with dodecanethiol for Schottky-diode chemical gas sensing devices
Uppsala universitet, Teknisk-naturvetenskapliga vetenskapsområdet, Tekniska sektionen, Institutionen för teknikvetenskaper, Fasta tillståndets fysik.
Uppsala universitet, Teknisk-naturvetenskapliga vetenskapsområdet, Tekniska sektionen, Institutionen för teknikvetenskaper, Fasta tillståndets fysik.
Visa övriga samt affilieringar
2017 (Engelska)Ingår i: Sensors and actuators. B, Chemical, ISSN 0925-4005, E-ISSN 1873-3077, Vol. 239, s. 455-461Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

Ultra-pure monolayer-capped gold nanoparticles for chemical gas sensing devices were prepared by a novel two-step process: a physical vapour deposition technique was first employed to make dispersed ultra-pure size-controlled gold nanoparticles, and this step was followed by a coating process for functionalization of the gold nanoparticles with an organic ligand, specifically dodecanethiol. X-ray photoelectron spectroscopy proved that the nano-assemblies had high purity. Chemical sensing devices based on these nano-assemblies showed Schottky-diode behaviour. We believe this is the first observation of Schottky-diodes fabricated from nanomaterials based on metallic nanoparticles. Gas sensing experiments demonstrated that these devices were suitable for detecting volatile organic compounds.

Ort, förlag, år, upplaga, sidor
2017. Vol. 239, s. 455-461
Nationell ämneskategori
Teknik och teknologier Materialkemi
Identifikatorer
URN: urn:nbn:se:uu:diva-302548DOI: 10.1016/j.snb.2016.07.182ISI: 000388951300056OAI: oai:DiVA.org:uu-302548DiVA, id: diva2:958089
Forskningsfinansiär
EU, FP7, Sjunde ramprogrammet, 267234Tillgänglig från: 2016-09-06 Skapad: 2016-09-06 Senast uppdaterad: 2017-09-28Bibliografiskt granskad
Ingår i avhandling
1. Thin films for indoor air monitoring: Measurements of Volatile Organic Compounds
Öppna denna publikation i ny flik eller fönster >>Thin films for indoor air monitoring: Measurements of Volatile Organic Compounds
2016 (Engelska)Doktorsavhandling, sammanläggning (Övrigt vetenskapligt)
Abstract [en]

Volatile organic compounds (VOCs) in the indoor air have adverse effects on the dwellers residing in a building or a vehicle. One of these effects is called sick building syndrome (SBS). SBS refers to situations in which the users of a building develop acute health effects and discomfort depending on the time they spend inside some buildings without having any specific illness. Furthermore, monitoring volatile organic compounds could lead to early diagnosis of specific illnesses through breath analysis. Among those VOCs formaldehyde, acetaldehyde can be listed.

In this thesis, VOC detecting thin film sensors have been investigated. Such sensors have been manufactured using semiconducting metal oxides, ligand activated gold nanoparticles and Graphene/TiO2 mixtures. Advanced gas deposition unit, have been used to produce NiO thin films and Au nanoparticles. DC magnetron sputtering has been used to produce InSnO and VO2 thin film sensors. Graphene/TiO2 sensors have been manufactured using doctor-blading.

While presenting the results, first, material characterization details are presented for each sensor, then, gas sensing results are presented. Morphologies, crystalline structures and chemical properties have been analyzed using scanning electron microscopy, X-ray diffraction and X-ray photo electron spectroscopy. Furthermore, more detailed analyses have been performed on NiO samples using extended X-ray absorption fine structure method and N2 adsorption measurements. Gas sensing measurements were focused on monitoring formaldehyde and acetaldehyde. However, responses ethanol and methane were measured in some cases to monitor selectivity. Graphene/TiO2 samples were used to monitor NO2 and NH3. For NiO thin film sensors and Au nano particles, fluctuation enhanced gas sensing is also presented in addition to conductometric measurements. 

Ort, förlag, år, upplaga, sidor
Uppsala: Acta Universitatis Upsaliensis, 2016. s. 78
Serie
Digital Comprehensive Summaries of Uppsala Dissertations from the Faculty of Science and Technology, ISSN 1651-6214 ; 1422
Nyckelord
gas sensor, thin film, adcanced gas depostion, sputter deposition, nickel oxide, gold nanoparticles, indium tin oxide, acetaldehyde, formaldehyde
Nationell ämneskategori
Nanoteknik
Identifikatorer
urn:nbn:se:uu:diva-302558 (URN)978-91-554-9683-8 (ISBN)
Disputation
2016-10-21, Room Å2001, Ångströmlaboratoriet, Lägerhyddsv 1, 13:15 (Engelska)
Opponent
Handledare
Forskningsfinansiär
EU, FP7, Sjunde ramprogrammet, 267234
Tillgänglig från: 2016-09-28 Skapad: 2016-09-06 Senast uppdaterad: 2016-10-14Bibliografiskt granskad

Open Access i DiVA

Fulltext saknas i DiVA

Övriga länkar

Förlagets fulltext

Personposter BETA

Topalian, ZarehGranqvist, Claes Göran

Sök vidare i DiVA

Av författaren/redaktören
Cindemir, UmutTopalian, ZarehGranqvist, Claes Göran
Av organisationen
Fasta tillståndets fysik
I samma tidskrift
Sensors and actuators. B, Chemical
Teknik och teknologierMaterialkemi

Sök vidare utanför DiVA

GoogleGoogle Scholar

doi
urn-nbn

Altmetricpoäng

doi
urn-nbn
Totalt: 2315 träffar
RefereraExporteraLänk till posten
Permanent länk

Direktlänk
Referera
Referensformat
  • apa
  • ieee
  • modern-language-association
  • vancouver
  • Annat format
Fler format
Språk
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Annat språk
Fler språk
Utmatningsformat
  • html
  • text
  • asciidoc
  • rtf