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High energy resolution off-resonant spectroscopy: A review
Institute of Physical Chemistry, Polish Academy of Sciences, Warsaw 01-224, Poland.
Department of Physics, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland.
Department of Physics, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland.
Physikalisch-Technische Bundesanstalt (PTB), Abbestr. 2-12, Berlin 10587,Germany.
Vise andre og tillknytning
2017 (engelsk)Inngår i: Spectrochimica Acta Part B - Atomic Spectroscopy, ISSN 0584-8547, E-ISSN 1873-3565, Vol. 136, nr Supplement C, s. 23-33Artikkel, forskningsoversikt (Fagfellevurdert) Published
Abstract [en]

We review the high energy resolution off-resonant spectroscopy (HEROS) technique. HEROS probes the unoccupied electronic states of matter in a single-shot manner thanks to the combination of off-resonant excitation around atomic core states using wavelength dispersive X-ray detection setups. In this review we provide a general introduction to the field of X-ray spectroscopy together with the specification of the available X-ray techniques and X-ray methodologies. Next, the theoretical description of the HEROS approach is introduced with a special focus on the derivation of the X-ray emission and X-ray absorption correspondence relation at off-resonant excitation conditions. Finally, a number of experimental HEROS reports are reviewed in the field of chemistry and material science. We emphasize the applicability of HEROS to pulsed X-ray sources, like X-ray free electron lasers, and support the review with experimental examples. The review is complemented with perspectives on and possible further applications of the HEROS technique to the field of X-ray science.

sted, utgiver, år, opplag, sider
2017. Vol. 136, nr Supplement C, s. 23-33
Emneord [en]
High energy resolution off-resonant X-ray spectroscopy, Time-resolved chemical speciation, Synchrotron and X-ray free electron laser radiation
HSV kategori
Forskningsprogram
Fysik med inriktning mot atom- molekyl- och kondenserande materiens fysik
Identifikatorer
URN: urn:nbn:se:uu:diva-337010DOI: 10.1016/j.sab.2017.08.002ISI: 000413608500004OAI: oai:DiVA.org:uu-337010DiVA, id: diva2:1167973
Tilgjengelig fra: 2017-12-19 Laget: 2017-12-19 Sist oppdatert: 2018-03-23bibliografisk kontrollert

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