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Valence double ionization electron spectra of CH3F, CH3Cl and CH3I
Univ Gothenburg, Dept Phys, Origovagen 6B, S-41296 Gothenburg, Sweden.
Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, South Parks Rd, Oxford OX1 3QZ, England;Univ Gothenburg, Dept Phys, Origovagen 6B, S-41296 Gothenburg, Sweden.
Univ Gothenburg, Dept Phys, Origovagen 6B, S-41296 Gothenburg, Sweden.
Univ Gothenburg, Dept Phys, Origovagen 6B, S-41296 Gothenburg, Sweden.
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2017 (English)In: Chemical Physics, ISSN 0301-0104, E-ISSN 1873-4421, Vol. 491, p. 42-47Article in journal (Refereed) Published
Abstract [en]

Valence double ionization electron spectra of the methyl fluoride, methyl chloride, and methyl iodide molecules have been recorded using a time-of-flight photoelectron-photoelectron coincidence technique. The spectra are interpreted by comparison with existing ionization data, Auger spectra, and theoretical calculations. The lowest double ionization energies have been found to be around 35.0 eV, 30.6 eV, and 26.67 eV for CH3F, CH3Cl and CH3I, respectively. These energies are also compared with the predictions and implications of an empirical rule for the lowest double ionization energy in molecules.

Place, publisher, year, edition, pages
2017. Vol. 491, p. 42-47
National Category
Atom and Molecular Physics and Optics Physical Chemistry
Identifiers
URN: urn:nbn:se:uu:diva-361064DOI: 10.1016/j.chemphys.2017.04.002ISI: 000404317700005OAI: oai:DiVA.org:uu-361064DiVA, id: diva2:1250058
Funder
Swedish Research CouncilKnut and Alice Wallenberg FoundationEU, FP7, Seventh Framework Programme, 312284Available from: 2018-09-21 Created: 2018-09-21 Last updated: 2018-09-21Bibliographically approved

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Karlsson, Leif

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