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Stimulated X-ray Raman scattering - a critical assessment of the building block of nonlinear X-ray spectroscopy
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2016 (English)In: Faraday discussions (Online), ISSN 1359-6640, E-ISSN 1364-5498, Vol. 194, 305-324 p.Article in journal (Refereed) Published
Abstract [en]

With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets.

Place, publisher, year, edition, pages
2016. Vol. 194, 305-324 p.
National Category
Atom and Molecular Physics and Optics
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URN: urn:nbn:se:uu:diva-312397DOI: 10.1039/C6FD00103CISI: 000392422200014PubMedID: 27711899OAI: oai:DiVA.org:uu-312397DiVA: diva2:1063211
Available from: 2017-01-09 Created: 2017-01-09 Last updated: 2017-03-10Bibliographically approved

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Mucke, MelanieAgåker, MarcusSåthe, ConnyRubensson, Jan-Erik
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Molecular and Condensed Matter PhysicsDepartment of Physics and Astronomy
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