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Substitution mechanism and structural study of Ag-doped LiCu2O2
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Structural Chemistry.
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Engineering Sciences, Solid State Physics. Karpov Inst Phys Chem, Dept Inorgan Mat, Ctr Mat Sci, Moscow 105064, Russia.ORCID iD: 0000-0002-7177-8464
Moscow Technol Univ, RU-119434 Moscow, Russia..
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Engineering Sciences, Solid State Physics.
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2017 (English)In: Solid State Sciences, ISSN 1293-2558, E-ISSN 1873-3085, Vol. 70, 36-40 p.Article in journal (Refereed) Published
Abstract [en]

Plate-like stoichiometric crystals of Ag-doped LiCu2O2 have been grown by slowly cooling Li2CO3 center dot 4(1 - x)CuO center dot 4xAgNO(3) (0 <= x <= 0.5) melts. X-ray single crystal diffraction has shown that the crystals are isostructural with LiCu2O2 and contain around 5 at % Ag (relative to the Cu atoms). The addition of silver to lithium cuprate crystals significantly increases their electrical conductivity but has little effect on the temperature behavior of their magnetic moment. The possible substitution mechanism is determined which supports Ag+ <-> Cu+, rather than Ag+ <-> Li+ in the Ag-doped LiCu2O2 crystals.

Place, publisher, year, edition, pages
ELSEVIER SCIENCE BV , 2017. Vol. 70, 36-40 p.
Keyword [en]
Doped lithium cuprate, X-ray diffraction, Twin crystal, Magnetic properties, Multiferroic
National Category
Physical Sciences Engineering and Technology
Identifiers
URN: urn:nbn:se:uu:diva-331223DOI: 10.1016/j.solidstatesciences.2017.06.004ISI: 000405485800005OAI: oai:DiVA.org:uu-331223DiVA: diva2:1150152
Funder
Swedish Research CouncilThe Swedish Foundation for International Cooperation in Research and Higher Education (STINT)
Available from: 2017-10-18 Created: 2017-10-18 Last updated: 2017-10-20Bibliographically approved

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Tellgren, RolandIvanov, SergeyNordblad, PerMathieu, Roland

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