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Transition dynamics in two-photon ionisation
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Theoretical Chemistry. Sorbonne Univ, UPMC Univ Paris 6, UMR 7614, Lab Chim Phys Matiere & Rayonnement, 4 Pl Jussieu, F-75231 Paris, France.;CNRS, UMR 7614, LCPMR, Paris, France.ORCID iD: 0000-0001-9418-6579
Sorbonne Univ, UPMC Univ Paris 6, UMR 7614, Lab Chim Phys Matiere & Rayonnement, 4 Pl Jussieu, F-75231 Paris, France.;CNRS, UMR 7614, LCPMR, Paris, France.;Ecole Normale Super, Dept Chem, 24 Rue Lhomond, F-75005 Paris, France.; Chim ParisTech, IRCP, 11 Rue Pierre & Marie Curie, F-75005 Paris, France.
Sorbonne Univ, UPMC Univ Paris 6, UMR 7614, Lab Chim Phys Matiere & Rayonnement, 4 Pl Jussieu, F-75231 Paris, France.;CNRS, UMR 7614, LCPMR, Paris, France.
Sorbonne Univ, UPMC Univ Paris 6, UMR 7614, Lab Chim Phys Matiere & Rayonnement, 4 Pl Jussieu, F-75231 Paris, France.;CNRS, UMR 7614, LCPMR, Paris, France.
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2017 (English)In: Journal of optics, ISSN 0150-536X, Vol. 19, no 11, article id 114011Article, review/survey (Refereed) Published
Abstract [en]

We review various aspects of photoemission dynamics in the case of two-photon ionisation. We first recall the definition of a transition phase specific to two-photon transitions. Numerical experiments on model atoms are used to show how the group delay associated with the transition phase is actually representative of the early dynamics of the detected photoelectron wave packets. Then we address the question of measuring these transition delays using a standard interferometric technique of experimental attosecond physics, so-called rabbit . Finally, we outline different reinterpretations of rabbit giving access to the more fundamental scattering dynamics affecting any photoemission processes.

Place, publisher, year, edition, pages
2017. Vol. 19, no 11, article id 114011
National Category
Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:uu:diva-336807DOI: 10.1088/2040-8986/aa8f56ISI: 000413718100001OAI: oai:DiVA.org:uu-336807DiVA, id: diva2:1167121
Available from: 2017-12-18 Created: 2017-12-18 Last updated: 2018-03-22Bibliographically approved

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Publisher's full texthttp://stacks.iop.org/2040-8986/19/i=11/a=114011

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Vacher, Morgane

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