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High energy resolution off-resonant spectroscopy: A review
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2017 (English)In: Spectrochimica Acta Part B - Atomic Spectroscopy, ISSN 0584-8547, E-ISSN 1873-3565, Vol. 136, no Supplement C, 23-33 p.Article in journal (Refereed) Published
Abstract [en]

We review the high energy resolution off-resonant spectroscopy (HEROS) technique. HEROS probes the unoccupied electronic states of matter in a single-shot manner thanks to the combination of off-resonant excitation around atomic core states using wavelength dispersive X-ray detection setups. In this review we provide a general introduction to the field of X-ray spectroscopy together with the specification of the available X-ray techniques and X-ray methodologies. Next, the theoretical description of the HEROS approach is introduced with a special focus on the derivation of the X-ray emission and X-ray absorption correspondence relation at off-resonant excitation conditions. Finally, a number of experimental HEROS reports are reviewed in the field of chemistry and material science. We emphasize the applicability of HEROS to pulsed X-ray sources, like X-ray free electron lasers, and support the review with experimental examples. The review is complemented with perspectives on and possible further applications of the HEROS technique to the field of X-ray science.

Place, publisher, year, edition, pages
2017. Vol. 136, no Supplement C, 23-33 p.
Keyword [en]
High energy resolution off-resonant X-ray spectroscopy, Time-resolved chemical speciation, Synchrotron and X-ray free electron laser radiation
National Category
Physical Chemistry
Research subject
Physics with spec. in Atomic, Molecular and Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-337010DOI: 10.1016/j.sab.2017.08.002OAI: oai:DiVA.org:uu-337010DiVA: diva2:1167973
Available from: 2017-12-19 Created: 2017-12-19 Last updated: 2017-12-19Bibliographically approved

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Sá, Jacinto

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