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One-Pot Tandem Photoredox and Cross-Coupling Catalysis with a Single Palladium Carbodicarbene Complex
Acad Sinica, Inst Chem, Taipei 11529, Taiwan;Natl Taiwan Univ, Dept Chem, Taipei 10161, Taiwan.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Physical Chemistry. Acad Sinica, Inst Chem, Taipei 11529, Taiwan.
Acad Sinica, Inst Chem, Taipei 11529, Taiwan.
Acad Sinica, Inst Chem, Taipei 11529, Taiwan.
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2018 (English)In: Angewandte Chemie International Edition, ISSN 1433-7851, E-ISSN 1521-3773, Vol. 57, no 17, p. 4622-4626Article in journal (Refereed) Published
Abstract [en]

The combination of conventional transition-metal-catalyzed coupling (2e(-) process) and photoredox catalysis (1e(-) process) has emerged as a powerful approach to catalyze difficult cross-coupling reactions under mild reaction conditions. Reported is a palladium carbodicarbene (CDC) complex that mediates both a Suzuki-Miyaura coupling and photoredox catalysis for C-N bond formation upon visible-light irradiation. These two catalytic pathways can be combined to promote both conventional transition-metal-catalyzed coupling and photoredox catalysis to mediate C-H arylation under ambient conditions with a single catalyst in an efficient one-pot process.

Place, publisher, year, edition, pages
2018. Vol. 57, no 17, p. 4622-4626
Keywords [en]
carbenes, cross-coupling, palladium, photocatalysis, reaction mechanisms
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:uu:diva-353200DOI: 10.1002/anie.201800951ISI: 000430165700030PubMedID: 29461658OAI: oai:DiVA.org:uu-353200DiVA, id: diva2:1217456
Available from: 2018-06-13 Created: 2018-06-13 Last updated: 2018-06-13Bibliographically approved

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Wang, Vincent Cho-Chien

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