A simplified approach to thermally activated delayed fluorescence (TADF) bipolar host polymersShow others and affiliations
2022 (English)In: Polymer Chemistry, ISSN 1759-9954, E-ISSN 1759-9962, Vol. 13, no 29, p. 4241-4248Article in journal (Refereed) Published
Abstract [en]
Organic Light Emitting Diodes (OLEDs) are a critical part of current consumer electronics, from mobile device displays to solid-state lighting. Thus demand for the development of industrially compatible OLED materials continues to increase. Herein, we introduce a series of solution-processible polymers incorporating a Thermally Activated Delayed Fluorescence (TADF) emitter and a host species in the side chain to finely adjust the charge transport properties. For balanced charge transport, a bipolar host polymer based on carbazole and alpha-carboline was investigated in addition to the commonly employed unipolar host mCP and an electron transporting version thereof. We demonstrate that the combination of unipolar co-hosts on one polymer chain can generate, with less synthetic effort, the same optoelectronic properties as a polymer carrying the corresponding bipolar host molecule as a pendant.
Place, publisher, year, edition, pages
Royal Society of Chemistry, 2022. Vol. 13, no 29, p. 4241-4248
National Category
Polymer Chemistry Nano Technology
Research subject
Engineering Science with specialization in Nanotechnology and Functional Materials
Identifiers
URN: urn:nbn:se:uu:diva-481279DOI: 10.1039/d2py00511eISI: 000822031700001OAI: oai:DiVA.org:uu-481279DiVA, id: diva2:1686242
Funder
Swedish Research Council, 2018-05973Australian Research Council, LP1701003872022-08-092022-08-092024-10-29Bibliographically approved