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A simplified approach to thermally activated delayed fluorescence (TADF) bipolar host polymers
Queensland Univ Technol QUT, Ctr Mat Sci, Sch Chem & Phys, 2 George St, Brisbane, Qld 4000, Australia..
Queensland Univ Technol QUT, Ctr Mat Sci, Sch Chem & Phys, 2 George St, Brisbane, Qld 4000, Australia..ORCID iD: 0000-0002-9690-2476
Queensland Univ Technol QUT, Ctr Mat Sci, Sch Chem & Phys, 2 George St, Brisbane, Qld 4000, Australia..
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Materials Science and Engineering, Nanotechnology and Functional Materials.ORCID iD: 0000-0002-9871-8015
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2022 (English)In: Polymer Chemistry, ISSN 1759-9954, E-ISSN 1759-9962, Vol. 13, no 29, p. 4241-4248Article in journal (Refereed) Published
Abstract [en]

Organic Light Emitting Diodes (OLEDs) are a critical part of current consumer electronics, from mobile device displays to solid-state lighting. Thus demand for the development of industrially compatible OLED materials continues to increase. Herein, we introduce a series of solution-processible polymers incorporating a Thermally Activated Delayed Fluorescence (TADF) emitter and a host species in the side chain to finely adjust the charge transport properties. For balanced charge transport, a bipolar host polymer based on carbazole and alpha-carboline was investigated in addition to the commonly employed unipolar host mCP and an electron transporting version thereof. We demonstrate that the combination of unipolar co-hosts on one polymer chain can generate, with less synthetic effort, the same optoelectronic properties as a polymer carrying the corresponding bipolar host molecule as a pendant.

Place, publisher, year, edition, pages
Royal Society of Chemistry, 2022. Vol. 13, no 29, p. 4241-4248
National Category
Polymer Chemistry Nano Technology
Research subject
Engineering Science with specialization in Nanotechnology and Functional Materials
Identifiers
URN: urn:nbn:se:uu:diva-481279DOI: 10.1039/d2py00511eISI: 000822031700001OAI: oai:DiVA.org:uu-481279DiVA, id: diva2:1686242
Funder
Swedish Research Council, 2018-05973Australian Research Council, LP170100387Available from: 2022-08-09 Created: 2022-08-09 Last updated: 2024-10-29Bibliographically approved

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Zaar, Felicia

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Cole, Cameron M.Zaar, FeliciaShaw, Paul E.Sonar, PrashantBarner-Kowollik, Christopher
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