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Molecular hysteresis in a rigid dinuclear ruthenium polypyridyl complex incorporating a ligand-bound ambidentate motif
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Photochemistry and Molecular Science.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Photochemistry and Molecular Science.
2008 (English)In: Inorganic Chemistry, ISSN 0020-1669, E-ISSN 1520-510X, Vol. 47, no 13, 5531-5533 p.Article in journal (Refereed) Published
Abstract [en]

Two alternative Ru-2(2+/3+) mixed-valence states are formed in the first dinuclear Ru complex with a ligand-bound ambidentate motif. The hysteretic electrochemical response follows a double-square scheme where the structure of the mixed-valence state depends on the previous isovalent state. The Ru3+ state of the pyrrolidine-substituted bisterpyridine unit is characterized by intense ligand-to-metal charge-transfer absorptions that provide a distinctive signature of the corresponding mixed-valence state.

Place, publisher, year, edition, pages
2008. Vol. 47, no 13, 5531-5533 p.
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Chemical Sciences
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URN: urn:nbn:se:uu:diva-110006DOI: 10.1021/ic800075bISI: 000257278000004OAI: oai:DiVA.org:uu-110006DiVA: diva2:275006
Available from: 2009-11-02 Created: 2009-11-02 Last updated: 2017-12-12Bibliographically approved

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Lomoth, Reiner

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