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Directing protonation in [FeFe] hydrogenase active site models by modifications in their second coordination sphere
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Photochemistry and Molecular Science, Molecular Biomimetics.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Biochemistry and Organic Chemistry.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Photochemistry and Molecular Science, Molecular Biomimetics.
2010 (English)In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 46, no 31, 5775-5777 p.Article in journal (Refereed) Published
Abstract [en]

Subtle changes in the second coordination sphere of [Cl(2)bdtFe(2)-(CO)(4)(Ph2P-CH2-X-CH2-PPh2)] (bdt = benzene-1,2-dithiolate, X = NCH3, NCH2CF3, CH2) that do not influence the electronic character of the Fe-2 center can however direct protonation to three different sites: the N in the bis-phosphane, the Fe-Fe bond or the bdt-S.

Place, publisher, year, edition, pages
2010. Vol. 46, no 31, 5775-5777 p.
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:uu:diva-135607DOI: 10.1039/c0cc00724bISI: 000280514500044OAI: oai:DiVA.org:uu-135607DiVA: diva2:375277
Available from: 2010-12-07 Created: 2010-12-07 Last updated: 2017-12-11Bibliographically approved

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Gogoll, Adolf

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