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Spatial Quantum Beats in Vibrational Resonant Inelastic Soft X-Ray Scattering at Dissociating States in Oxygen
MAX-lab, Lund University, Box 118, S-221 00 Lund, Sweden.
Department of Theoretical Chemistry and Biology, School of Biotechnology, Royal Institute of Technology, S-106 91 Stockholm, Sweden.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Soft X-Ray Physics.
Department of Theoretical Chemistry and Biology, School of Biotechnology, Royal Institute of Technology, S-106 91 Stockholm, Sweden.
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2011 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 106, no 15, 153004-1-153004-4 p.Article in journal (Refereed) Published
Abstract [en]

Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1 sigma(g) -> 3 sigma(u) resonance in gas-phase O-2 show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.

Place, publisher, year, edition, pages
2011. Vol. 106, no 15, 153004-1-153004-4 p.
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Physical Sciences
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URN: urn:nbn:se:uu:diva-153939DOI: 10.1103/PhysRevLett.106.153004ISI: 000289525300005OAI: oai:DiVA.org:uu-153939DiVA: diva2:418585
Available from: 2011-05-23 Created: 2011-05-23 Last updated: 2017-12-11Bibliographically approved

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Hennies, Franz

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