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Mechanism of hydrogen transfer to imines from a hydroxycyclopentadienyl ruthenium hydride. Support for a stepwise mechanism.
2004 (English)In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, no 23, 2748-2749 p.Article in journal (Refereed) Published
Abstract [en]

The negligible double kinetic deuterium isotope effect (kHH/kDD = 1.05) in the reaction where [2,3,4,5-Ph4(η5-C4COH)]Ru(CO)2H (2) transfers a hydride and a proton to N-phenyl-[1-(4-methoxyphenyl)ethylidene]amine (4) indicates that no bond to hydrogen is broken or formed in the rate-detg. step. [on SciFinder(R)]

Place, publisher, year, edition, pages
2004. no 23, 2748-2749 p.
Keyword [en]
hydrogen transfer imine hydroxycyclopentadienylruthenium hydride stepwise mechanism
National Category
Natural Sciences
Identifiers
URN: urn:nbn:se:uu:diva-174523DOI: 10.1039/b410698aOAI: oai:DiVA.org:uu-174523DiVA: diva2:527596
Note
CAPLUS AN 2004:1037547(Journal)Available from: 2012-05-21 Created: 2012-05-21 Last updated: 2017-12-07

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Samec, Joseph S. M.

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