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Enantioselective addition of aldehydes to amines via combined catalytic biomimetic oxidation and organocatalytic C-C bond formation.
2005 (English)In: Tetrahedron Letters, ISSN 0040-4039, E-ISSN 1359-8562, Vol. 46, no 23, 3965-3968 p.Article in journal (Refereed) Published
Abstract [en]

The biomimetic catalytic enantioselective addn. of aldehydes to amines is reported. This was accomplished by combining biomimetic coupled catalytic aerobic oxidn. of amines involving ruthenium-induced dehydrogenation and organocatalytic asym. Mannich reactions. The one-pot reactions furnished β-amino aldehyde and α-amino acid derivs. in high yields with excellent chemoselectivity and enantioselectivity. [on SciFinder(R)]

Place, publisher, year, edition, pages
2005. Vol. 46, no 23, 3965-3968 p.
Keyword [en]
amine ruthenium hydroquinone cobalt biomimetic oxidn propanal addn proline, amino aldehyde asym prepn redn, alc amino asym prepn, ruthenium hydroquinone cobalt biomimetic oxidn catalyst, proline asym Mannich reaction catalyst
National Category
Natural Sciences
Identifiers
URN: urn:nbn:se:uu:diva-174521DOI: 10.1016/j.tetlet.2005.04.047OAI: oai:DiVA.org:uu-174521DiVA: diva2:527597
Note
CAPLUS AN 2005:411368(Journal)Available from: 2012-05-21 Created: 2012-05-21 Last updated: 2017-12-07

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Samec, Joseph S. M.

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