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Site-selective resonant Auger spectroscopy of iso-dichloroethylene at the carbon K-edge
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Surface and Interface Science.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Surface and Interface Science.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Surface and Interface Science.
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2012 (English)In: Journal of Electron Spectroscopy and Related Phenomena, ISSN 0368-2048, E-ISSN 1873-2526, Vol. 185, no 8-9, 252-258 p.Article in journal (Refereed) Published
Abstract [en]

This study focuses on the two C1s-to-LUMO (lowest unoccupied molecular orbital) excitations of the iso-dichloroethylene (H2C=CCl2) and the subsequent Auger decay. We investigate the effect of the two different carbon core excitations on the population of the cation produced after electronic relaxation. The resonant Auger spectra are interpreted by comparison to the valence shells photoionization spectrum and with the help of theoretical calculations. Several consequences of the core-hole localization on the electronic decay are observed. In particular, the resonant excitation of the C1s(CH2) to the LUMO leads to a large intensity increase in the region of the first satellite state, whereas no dramatic changes are observed for the C1s(CCl2) excitation.

Place, publisher, year, edition, pages
2012. Vol. 185, no 8-9, 252-258 p.
Keyword [en]
Resonant Auger, Nuclear dynamics, Mulliken's population analysis
National Category
Physical Sciences
Identifiers
URN: urn:nbn:se:uu:diva-182767DOI: 10.1016/j.elspec.2012.06.005ISI: 000308627700010OAI: oai:DiVA.org:uu-182767DiVA: diva2:561207
Available from: 2012-10-17 Created: 2012-10-15 Last updated: 2017-12-07Bibliographically approved

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Piancastelli, Maria Novella

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