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Formation and decay of core-orbital vacancies in the water molecule
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Molecular and condensed matter physics.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Molecular and condensed matter physics.
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2013 (English)In: Chemical Physics Letters, ISSN 0009-2614, E-ISSN 1873-4448, Vol. 558, 82-87 p.Article in journal (Refereed) Published
Abstract [en]

Primary steps in the interaction of high energy photons with water creating multiply ionised products are examined experimentally and theoretically. Double Auger decay from a 1s-hole state populates triply ionised states between 80 and 140 eV binding energy. Ejection of one 1s electron and one valence electron gives states around 570 eV which decay to triply ionised states between 75 and 110 eV. Nuclear motion in these states competes with Auger decay and substantially modifies the final state spectra. The double core-hole state from ionisation of both 1s electrons is found at 1171 +/- 1 eV and calculated at 1170.85 eV. 

Place, publisher, year, edition, pages
2013. Vol. 558, 82-87 p.
National Category
Natural Sciences Engineering and Technology
Research subject
Engineering Science with specialization in Solid State Physics
Identifiers
URN: urn:nbn:se:uu:diva-196532DOI: 10.1016/j.cplett.2012.11.094ISI: 000314660600016OAI: oai:DiVA.org:uu-196532DiVA: diva2:610859
Available from: 2013-03-13 Created: 2013-03-11 Last updated: 2017-12-06Bibliographically approved

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Mucke, MelanieEland, John H. D.Lebrun, DelphineFeifel, Raimund

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