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Electronic-structure investigation of CeB6 by means of soft-x-ray scattering
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics.
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2001 (English)In: Physical Review B Condensed Matter, ISSN 0163-1829, E-ISSN 1095-3795, Vol. 63, no 7, 075101- p.Article in journal (Refereed) Published
Abstract [en]

The electronic structure of the heavy fermion compound CeB6 is probed by resonant inelastic soft-x-ray scattering using photon energies across the Ce 3d and 4dabsorption edges. The hybridization between the localized 4f orbitals and the delocalized valence-band states is studied by identifying the different spectral contributions from inelastic Raman scattering and normal fluorescence. Pronounced energy-loss structures are observed below the elastic peak at both the 3d and 4dthresholds. The origin and character of the inelastic scattering structures are discussed in terms of charge-transfer excitations in connection to the dipole allowed transitions with 4f character. Calculations within the single-impurity Anderson model with full multiplet effects are found to yield consistent spectral functions to the experimental data.

Place, publisher, year, edition, pages
2001. Vol. 63, no 7, 075101- p.
Keyword [en]
RARE-EARTH HEXABORIDES; HIGH-RESOLUTION; PHOTOEMISSION SPECTROSCOPY; RESONANT PHOTOEMISSION; EMISSION SPECTRA; SINGLE-CRYSTALS; SYSTEMS; EXCITATIONS; SURFACE; CERIUM
National Category
Physical Sciences
Identifiers
URN: urn:nbn:se:uu:diva-37235DOI: 10.1103/PhysRevB.63.075101OAI: oai:DiVA.org:uu-37235DiVA: diva2:65134
Available from: 2006-11-15 Created: 2006-11-15 Last updated: 2017-12-06Bibliographically approved

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Magnuson, MartinNordgren, Joseph

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