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A review of molecular effects in gas-phase KL X-ray emission
UPMC Univ Paris 06, UMR 7614, Lab Chim Phys Mat & Rayonnement, Paris.; CNRS, UMR 7614, Lab Chim Phys Mat & Rayonnement, Paris.
UPMC Univ Paris 06, UMR 7614, Lab Chim Phys Mat & Rayonnement, Paris.; CNRS, UMR 7614, Lab Chim Phys Mat & Rayonnement, Paris.
UPMC Univ Paris 06, UMR 7614, Lab Chim Phys Mat & Rayonnement, Paris.; CNRS, UMR 7614, Lab Chim Phys Mat & Rayonnement, Paris.
Univ Nevada, Dept Chem, Las Vegas.
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2013 (English)In: Journal of Electron Spectroscopy and Related Phenomena, ISSN 0368-2048, E-ISSN 1873-2526, Vol. 188, p. 53-61Article, review/survey (Refereed) Published
Abstract [en]

The unique capabilities of resonant inelastic X-ray scattering (RIXS) to provide a deep insight into molecular dynamics following core excitation are reviewed here. Characteristic features of molecular X-ray emission are experimentally observed and theoretically interpreted. Some of our most significant results on molecular dynamics following deep core excitation are presented. In particular, we provide several examples of nuclear dynamics on the femtosecond or subfemtosecond time scale; line-narrowing effects related to the quenching of vibrational structure due to parallelism of intermediate and final state curves; anomalous line dispersion across a resonance, which is due to core-hole lifetime effects; spin–orbit-state populations derived from polarized RIXS experiments. We also show how to connect the RIXS results to the general chemical properties of the investigated systems.

Place, publisher, year, edition, pages
2013. Vol. 188, p. 53-61
Keyword [en]
Gas phase, Molecular dynamics, Polarization, Resonant inelastic X-ray scattering, Spectroscopy
National Category
Theoretical Chemistry Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-217759DOI: 10.1016/j.elspec.2012.11.007ISI: 000324008900009OAI: oai:DiVA.org:uu-217759DiVA, id: diva2:693597
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Times Cited: 0 Si

Available from: 2014-02-04 Created: 2014-02-04 Last updated: 2018-04-06

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Piancastelli, Maria Novella

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