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Role of resonant inelastic X-ray scattering in high-resolution core-level spectroscopy of actinide materials
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Molecular and condensed matter physics.
2014 (English)In: Journal of Electron Spectroscopy and Related Phenomena, ISSN 0368-2048, E-ISSN 1873-2526, Vol. 194, 27-36 p.Article in journal (Refereed) Published
Abstract [en]

This paper provides a brief overview of applications of advanced X-ray spectroscopic techniques that take advantage of the resonant inelastic X-ray scattering (RIXS) in the hard and tender X-ray range and have recently become available for studying the electronic structure of actinides. We focus here on the high-energy-resolution X-ray absorption near edge structure (XANES) and core-to-core and core-to-valence RIXS spectroscopies at the U L and M edges of uranium compounds. The spectral features are analyzed using a number of theoretical methods, such as the Anderson impurity model, density functional theory in the local density approximation with an added Coulomb interaction (LDA + U), and full multiple scattering (FEFF) and ab initio finite difference method near-edge structure (FDMNES) codes. In connection with presented results, the capabilities and limitations of the experimental techniques and theoretical methods are discussed. (C) 2014 Elsevier B.V. All rights reserved.

Place, publisher, year, edition, pages
2014. Vol. 194, 27-36 p.
Keyword [en]
Actinides, X-ray spectroscopy, XANES, RIXS, Electronic structure
National Category
Physical Sciences
Identifiers
URN: urn:nbn:se:uu:diva-230526DOI: 10.1016/j.elspec.2014.01.016ISI: 000339040000006OAI: oai:DiVA.org:uu-230526DiVA: diva2:741655
Available from: 2014-08-28 Created: 2014-08-26 Last updated: 2017-12-05Bibliographically approved

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Kvashnin, YaroslavButorin, Sergei

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