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Suppression of the molecular ultra-fast dissociation in bromomethane clusters
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Molecular and condensed matter physics.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Molecular and condensed matter physics.ORCID iD: 0000-0002-9188-9604
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy.
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2014 (English)In: Journal of Chemical Physics, ISSN 0021-9606, E-ISSN 1089-7690, Vol. 141, 224305- p.Article in journal (Refereed) Published
Abstract [en]

We address the influence of clustering on the ultra-fast dissociation of bromomethane. Valence and core photo-electron spectroscopy, partial electron yield absorption, and resonant Auger spectroscopy have been used together with ab initio calculations to investigate the properties of the ultra-fast dissociation. The ratio of ultra-fast dissociation of molecules in clusters as compared to free molecules is determined to be significantly reduced. We propose partial delocalization of the excited electronic state as being responsible for this behavior.

Place, publisher, year, edition, pages
AIP, 2014. Vol. 141, 224305- p.
National Category
Physical Sciences
Research subject
Physics with spec. in Atomic, Molecular and Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-241035DOI: 10.1063/1.4903455ISI: 000346272800023OAI: oai:DiVA.org:uu-241035DiVA: diva2:777519
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UBJL
Funder
Swedish Research Council
Available from: 2015-01-08 Created: 2015-01-08 Last updated: 2017-12-05Bibliographically approved

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Lindblad, AndreasSvensson, SvanteBjörneholm, Olle

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