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Determination of catalytic reaction mechanisms by isotopic frequency response.
2012 (English)In: The Analyst, ISSN 0003-2654, E-ISSN 1364-5528, Vol. 137, no 22, 5374-81 p.Article in journal (Refereed) Published
Abstract [en]

Efficient catalysts are of extraordinary importance for the development of efficient chemical processes as well as applications such as energy storage. Rational development of catalysts requires a mechanistic understanding of the catalytic reaction. Since steady-state investigations are insufficient to gain mechanistic understanding, transient methods such as SSITKA and frequency response have been developed. In this paper we provide a theoretical basis for a frequency response method based on variations in the isotopic composition of the reactant. This approach is particularly useful, since it permits transient investigations under quasi-steady state conditions and because the response is linear.

Place, publisher, year, edition, pages
2012. Vol. 137, no 22, 5374-81 p.
National Category
Physical Chemistry
Identifiers
URN: urn:nbn:se:uu:diva-252499DOI: 10.1039/c2an35903kPubMedID: 23034591OAI: oai:DiVA.org:uu-252499DiVA: diva2:810904
Available from: 2015-05-08 Created: 2015-05-07 Last updated: 2017-12-04

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