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Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Molecular and condensed matter physics.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Molecular and condensed matter physics.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy.
Uppsala University, Disciplinary Domain of Medicine and Pharmacy, Faculty of Pharmacy, Department of Pharmacy.
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2015 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 114, no 13, 133001Article in journal (Refereed) Published
Abstract [en]

Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.

Place, publisher, year, edition, pages
2015. Vol. 114, no 13, 133001
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Physical Sciences
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URN: urn:nbn:se:uu:diva-251994DOI: 10.1103/PhysRevLett.114.133001ISI: 000352073600001PubMedID: 25884123OAI: oai:DiVA.org:uu-251994DiVA: diva2:811118
Available from: 2015-05-11 Created: 2015-04-28 Last updated: 2017-12-04Bibliographically approved

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Rubensson, Jan-ErikSöderström, JohanBinggeli, ChristianGråsjö, JohanAndersson, Joakim

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Molecular and condensed matter physicsDepartment of Physics and AstronomyDepartment of Pharmacy
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