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Water oxidation catalysed by a mononuclear CoII polypyridine complex; possible reaction intermediates and the role of the chloride ligand
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Molecular Biomimetics.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Molecular Biomimetics.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Molecular Biomimetics.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Molecular Biomimetics.ORCID iD: 0000-0001-7643-302X
2015 (English)In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 51, no 66, 13074-13077 p.Article in journal (Refereed) Published
Abstract [en]

A mononuclear cobalt(II) complex as a homogeneous molecular catalyst for photochemically, electrochemically and chemically induced oxygen evolution reactions is presented. Experimental evidence points towards the presence of a chloride ligand at the cobalt centre throughout the catalytic cycle, and the temporary detachment of a pyridine ligand to open a coordination site for substrate binding.

Place, publisher, year, edition, pages
2015. Vol. 51, no 66, 13074-13077 p.
National Category
Inorganic Chemistry
Identifiers
URN: urn:nbn:se:uu:diva-257686DOI: 10.1039/c5cc04148aISI: 000359151100003OAI: oai:DiVA.org:uu-257686DiVA: diva2:840230
Funder
Knut and Alice Wallenberg FoundationSwedish Energy AgencySwedish Research Council
Available from: 2015-07-07 Created: 2015-07-07 Last updated: 2017-12-04Bibliographically approved

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Das, BiswanathOrthaber, AndreasOtt, SaschaThapper, Anders

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