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Synthesis and Photophysics of One Mononuclear Mn(III) and One Dinuclear Mn(III,III) Complex Covalently Linked to a Ruthenium(II) Tris(bipyridyl) Complex
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Physical Chemistry.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Molecular Biomimetics.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Molecular Biomimetics.
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2003 (English)In: Inorganic Chemistry, Vol. 42, 7502-7511 p.Article in journal (Refereed) Published
Abstract [en]

The preparation of donor (D)-photosensitizer (S) arrays, consisting of a manganese complex as D and a ruthenium tris(bipyridyl) complex as S has been pursued. Two new ruthenium complexes containing coordinating sites for one (2a) and two manganese ions (3a) were prepared in order to provide models for the donor side of photosystem II in green plants. The manganese coordinating site consists of bridging and terminal phenolate as well as terminal pyridyl ligands. The corresponding ruthenium-manganese complexes, a manganese monomer 2b and dimer 3b, were obtained. For the dimer 3b, our data suggest that intramolecular electron transfer from manganese to photogenerated ruthenium(III) is fast, k(ET) > 5 x 10(7) s(-1).

Place, publisher, year, edition, pages
American Chemical Society , 2003. Vol. 42, 7502-7511 p.
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Chemical Sciences
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URN: urn:nbn:se:uu:diva-271357DOI: 10.1021/ic0344822OAI: oai:DiVA.org:uu-271357DiVA: diva2:891790
Available from: 2016-01-07 Created: 2016-01-07 Last updated: 2016-01-07

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Magnuson, AnnStyring, Stenbjörn

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