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  • 1.
    Hattori, Yocefu
    et al.
    Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Physical Chemistry.
    Abdellah, Mohamed
    Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Physical Chemistry. South Valley Univ, Qena Fac Sci, Dept Chem, Qena 83523, Egypt.
    Meng, Jie
    Tech Univ Denmark, Dept Chem, DK-2800 Lyngby, Denmark.
    Zheng, Kaibo
    Tech Univ Denmark, Dept Chem, DK-2800 Lyngby, Denmark;Lund Univ, Chem Phys & NanoLund, Box 124, S-22100 Lund, Sweden.
    Sá, Jacinto
    Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Physical Chemistry. Polish Acad Sci, Inst Phys Chem, PL-01224 Warsaw, Poland.
    Simultaneous Hot Electron and Hole Injection upon Excitation of Gold Surface Plasmon2019In: Journal of Physical Chemistry Letters, ISSN 1948-7185, E-ISSN 1948-7185, Vol. 10, no 11, p. 3140-3146Article in journal (Refereed)
    Abstract [en]

    We have successfully investigated the simultaneous injection of hot electrons and holes upon excitation of gold localized surface plasmon resonance (LSPR). The studies were performed on all-solid-state plasmonic system composed of titanium dioxide (TiO2)/poly(3,4-ethylenedioxythiophene) :poly(styrenesulfonic acid) (PEDOT:PSS) p-n junctions with gold nanoparticles (Au NPs). The study revealed that both charge carriers are transferred within 200 fs to the respective charge acceptors, exhibiting a free carrier transport behavior. We also confirmed that the transfer of charge carriers are accompanied by change in the initial relaxation dynamics of Au NPs.

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