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  • 1.
    Azimi Mousolou, Vahid
    et al.
    School of Computer Science, Physics and Mathematics, Linnaeus Univ., Sweden.
    Canali, Carlo M.
    Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Physical and Analytical Chemistry, Theoretical Chemistry. School of Computer Science, Physics and Mathematics, Linnaeus Univ., Sweden.
    Sjöqvist, Erik
    Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Theoretical Chemistry.
    Universal Non-adiabatic Holonomic Gates in Quantum Dots and Single-Molecule Magnets2014In: New Journal of Physics, ISSN 1367-2630, E-ISSN 1367-2630, Vol. 16, article id 013029Article in journal (Refereed)
    Abstract [en]

    Geometric manipulation of a quantum system offers a method for fast, universal, and robust quantum information processing. Here, we propose a scheme for universal all-geometric quantum computation using non-adiabatic quantum holonomies. We propose three different realizations of the scheme based on an unconventional use of quantum dot and single-molecule magnet devices, which offer promising scalability and robust efficiency. 

  • 2. Navizet, Isabelle
    et al.
    Liu, Ya-Jun
    Ferre, Nicolas
    Roca Sanjuán, Daniel
    Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Physical and Analytical Chemistry, Theoretical Chemistry.
    Lindh, Roland
    Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Physical and Analytical Chemistry, Theoretical Chemistry.
    The Chemistry of Bioluminescence: An Analysis of Chemical Functionalities2011In: ChemPhysChem, ISSN 1439-4235, E-ISSN 1439-7641, Vol. 12, no 17, p. 3064-3076Article, review/survey (Refereed)
    Abstract [en]

    Firefly luciferase is one of the most studied bioluminescent systems, both theoretically and experimentally. Herein we review the current understanding of the bioluminescent process from a chemical functionality perspective based on those investigations. Three key components are emphasized: the chemiluminophore, the electron-donating fragment, and how these are affected by the substrateenzyme interaction. The understanding is based on details of how the peroxide ?O?O? bond supports the production of electronically excited products and how the charge-transfer (CT) mechanism, with the aid of an electron-donating group, lowers the activation barrier to support a reaction occurs in living organisms. For the substrateenzyme complex it is demonstrated that the enzyme can affect the hydrogen-bonding around the CT-controlling group, resulting in a mechanism for color modulation. Finally, we analyse other luciferinluciferase systems and compare them to the key chemical functionalities of the fragments of the luciferinluciferase complex with respect to similarities and differences.

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