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The work in this dissertation is devoted to tailoring and studying magnetic properties of epitaxial metal/oxide heterostructures. The aim is to understand the fundamental principles governing these properties and how they affect each other. The acquired knowledge can prove useful for the development of future spintronic devices. A variety of experimental techniques is used to fabricate and characterize the epitaxial structures. For fabrication, a combination of direct-current and radio-frequency sputtering is used, whereas x-ray reflectivity and diffraction measurements are the main tools for the structural characterization of the heterostructures. The magnetic characterization of these structures is done by a combination of longitudinal magneto-optical Kerr-effect measurements, Kerr-microscopy and polarized neutron reflectometry. 

First, it is shown how strain affects the magnetic properties of metal/oxide heterostructures by comparing Fe/MgO and Fe/MgAl₂O₄ superlattices. Subsequently, an antiferromagnetic interlayer exchange coupling in  Fe/MgO superlattices is revealed and attributed to a spin-polarized-tunneling mechanism. The coupling strength can be tuned by changing the MgO thickness leading to the stabilization of different remanent states as well as to different reversal mechanisms. It is shown that the interlayer exchange coupling in Fe/MgO superlattices is a consequence of two distinct components. These components can be interpreted as beyond-nearest-neighbor interactions and a contribution arising from the total thickness of the heterostructures.

The interlayer exchange coupling is further investigated via temperature dependent magnetization measurements. It is shown that different remanent states and reversal mechanisms occur at different temperatures. Furthermore, a large increase in interlayer exchange coupling strength with reduced temperature is revealed. 

Finally, it is shown that Fe₈₄Cu₁₆/MgO superlattices exhibit a reduced magnetocrystalline anisotropy and interlayer exchange coupling strength, as compared to pure Fe/MgO superlattices. Patterning such Fe₈₄Cu₁₆/MgO superlattices in circular islands leads to an increased saturation field with decreasing island diameter.