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Ultrafast terahertz magnetometry
Univ Bielefeld, Fak Phys, Univ Str 25, D-33615 Bielefeld, Germany.;Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany..
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory.ORCID iD: 0000-0002-8524-819X
Univ Shanghai Sci & Technol, Terahertz Technol Innovat Res Inst, JunGong Rd 516, Shanghai 200093, Peoples R China..
Swiss Fed Inst Technol, Dept Mat, Honggerbergring 64, CH-8093 Zurich, Switzerland..
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2020 (English)In: Nature Communications, E-ISSN 2041-1723, Vol. 11, no 1, article id 4247Article in journal (Refereed) Published
Abstract [en]

A material's magnetic state and its dynamics are of great fundamental research interest and are also at the core of a wide plethora of modern technologies. However, reliable access to magnetization dynamics in materials and devices on the technologically relevant ultrafast timescale, and under realistic device-operation conditions, remains a challenge. Here, we demonstrate a method of ultrafast terahertz (THz) magnetometry, which gives direct access to the (sub-)picosecond magnetization dynamics even in encapsulated materials or devices in a contact-free fashion, in a fully calibrated manner, and under ambient conditions. As a showcase for this powerful method, we measure the ultrafast magnetization dynamics in a laser-excited encapsulated iron film. Our measurements reveal and disentangle distinct contributions originating from (i) incoherent hot-magnon-driven magnetization quenching and (ii) coherent acoustically-driven modulation of the exchange interaction in iron, paving the way to technologies utilizing ultrafast heat-free control of magnetism. High sensitivity and relative ease of experimental arrangement highlight the promise of ultrafast THz magnetometry for both fundamental studies and the technological applications of magnetism.

Place, publisher, year, edition, pages
NATURE PUBLISHING GROUP , 2020. Vol. 11, no 1, article id 4247
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-421525DOI: 10.1038/s41467-020-17935-6ISI: 000567537300006PubMedID: 32843645OAI: oai:DiVA.org:uu-421525DiVA, id: diva2:1474756
Funder
Swedish Research CouncilKnut and Alice Wallenberg Foundation, 2015.0060Swedish National Infrastructure for Computing (SNIC)Available from: 2020-10-09 Created: 2020-10-09 Last updated: 2023-03-28Bibliographically approved

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Maldonado, PabloOppeneer, Peter M.

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