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Theory of out-of-equilibrium electron and phonon dynamics in metals after femtosecond laser excitation
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory. Free Univ Berlin, Dept Phys, Arnimallee 14, D-14195 Berlin, Germany.;Free Univ Berlin, Dahlem Ctr Complex Quantum Syst, Arnimallee 14, D-14195 Berlin, Germany..
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory. Free Univ Berlin, Dept Phys, Arnimallee 14, D-14195 Berlin, Germany..ORCID iD: 0000-0002-9069-2631
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory.
2020 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 102, no 21, article id 214305Article in journal (Refereed) Published
Abstract [en]

The dynamics of electrons and phonons in metals upon laser excitation are often described by the two-temperature model, which assumes that both subsystems are individually in thermal equilibrium. However, recent experiments show that this description is not sufficient to describe the out-of-equilibrium dynamics on ultrashort timescales. Here, assuming a thermalized electronic system, we extend and apply a parameter-free microscopic out-of-equilibrium model to describe the ultrafast laser-induced phonon and electron temperature dynamics of various metallic systems such as gold, aluminum, iron, nickel, and cobalt. We report strong deviations from the two-temperature model on the picosecond timescale for all the materials studied, even for those where the assumption of separate thermal equilibrium seemed less restrictive, like in gold. Furthermore, we demonstrate the importance of the mode dependence of the electron-phonon coupling for the relaxation process and reveal the significance of this channel in the lattice equilibration.

Place, publisher, year, edition, pages
AMER PHYSICAL SOC , 2020. Vol. 102, no 21, article id 214305
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Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-431842DOI: 10.1103/PhysRevB.102.214305ISI: 000600275000004OAI: oai:DiVA.org:uu-431842DiVA, id: diva2:1519244
Funder
Swedish Research CouncilKnut and Alice Wallenberg Foundation, 2015.0060Swedish National Infrastructure for Computing (SNIC)German Research Foundation (DFG), RI 2891/1-1German Research Foundation (DFG), RI 2891/2-1German Research Foundation (DFG), TRR 227Available from: 2021-01-18 Created: 2021-01-18 Last updated: 2021-01-18Bibliographically approved

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Ritzmann, UlrikeOppeneer, Peter M.Maldonado, Pablo

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