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2D crystal structure and anisotropic magnetism of GdAu6.75-xAl0.5+x (x approximate to 0.54)
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Materials Science and Engineering, Solid State Physics.ORCID iD: 0000-0001-9701-1766
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström.ORCID iD: 0000-0003-1804-8259
Augsburg Univ, Inst Phys, D-86159 Augsburg, Germany..
Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden..
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2022 (English)In: Scientific Reports, E-ISSN 2045-2322, Vol. 12, article id 13141Article in journal (Refereed) Published
Abstract [en]

Exploration of the gold-rich part of the ternary Gd-Au-Al system afforded the intermetallic compound GdAu6.75-xAl0.5+x (x approximate to 0.54) which was structurally characterized by single crystal X-ray diffraction (Pnma, a = 18.7847(4) angstrom, b = 23.8208(5) angstrom, c = 5.3010(1) angstrom). GdAu6.75-xAl0.5+x crystallizes in a previously unknown structure type featuring layers of Gd-2(Au, Al)(29) and Gd-2(Au, Al)(28) clusters which are arranged as in a close-packing parallel to the ac plane. The Gd substructure corresponds to slightly corrugated 3(6) nets (d(Gd-Gd) = 5.30-5.41 angstrom) which are stacked on top of each other along the b direction with alternating short (5.4, 5.6 angstrom, within layers) and long distances (6.4 angstrom, between layers). The title compound has been discussed with respect to a quasicrystal approximant (1/1 AC) GdAu5.3Al in the same system. The magnetic properties of GdAu6.75-xAl0.5+x were found to be reminiscent to those of some ternary ACs, with sharp peaks in the temperature dependent magnetization, and metamagnetic-like transitions. The material becomes antiferromagnetic below 25 K; magnetometry results suggest that the antiferromagnetic state is composed of ferromagnetic ac planes, coupled antiferromagnetically along the b direction.

Place, publisher, year, edition, pages
Springer Nature Springer Nature, 2022. Vol. 12, article id 13141
National Category
Materials Chemistry
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URN: urn:nbn:se:uu:diva-482044DOI: 10.1038/s41598-022-17068-4ISI: 000834790800028PubMedID: 35907933OAI: oai:DiVA.org:uu-482044DiVA, id: diva2:1688474
Funder
Knut and Alice Wallenberg Foundation, KAW 2018.0019Swedish Research CouncilOlle Engkvists stiftelse, 184-546Available from: 2022-08-18 Created: 2022-08-18 Last updated: 2024-01-15Bibliographically approved

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Joshi, Deep C.Gebresenbut, Girma HailuNordblad, PerMathieu, Roland

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