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Examination of the critical behavior and magnetocaloric effect of the ferromagnetic Gd-Au-Si quasicrystal approximants
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Materials Science and Engineering, Solid State Physics.ORCID iD: 0000-0002-2671-324x
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Structural Chemistry.ORCID iD: 0000-0003-1804-8259
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Structural Chemistry.ORCID iD: 0000-0002-9349-1077
Stockholm Univ, Dept Mat & Environm Chem, S-10691 Stockholm, Sweden..
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2022 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 106, no 17, article id 174405Article in journal (Refereed) Published
Abstract [en]

We investigate the critical behavior and magnetocaloric effects of the Gd-Au-Si (GAS) ferromagnetic quasicrystal approximants, Gd13.7Au72.7Si13.6 [referred to as GAS(0)] and Gd15.4Au68.6Si16.0 [GAS(100)]. The former is a conventional Tsai-type 1/1 approximant crystal, while the latter has a slightly different atomic decoration from the Tsai type (thus referred to as “pseudo-Tsai” type). Their critical exponents at the ferromagnetic transitions are close to those of the mean-field theory. Both GAS systems exhibit an interesting magnetic-field dependence of the specific heat, which is reflected in the behavior of their magnetocaloric effect (MCE). The MCE is characterized by an adiabatic cooling (heating) effect over a relatively broad temperature range below ∼30 K, which stems from a broad feature in the specific heat.

Place, publisher, year, edition, pages
American Physical Society, 2022. Vol. 106, no 17, article id 174405
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Condensed Matter Physics
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URN: urn:nbn:se:uu:diva-490382DOI: 10.1103/PhysRevB.106.174405ISI: 000885458200002OAI: oai:DiVA.org:uu-490382DiVA, id: diva2:1719293
Funder
Knut and Alice Wallenberg Foundation, KAW 2018.0019Swedish Research Council, 2021-04360Carl Tryggers foundation , CTS 19:235Available from: 2022-12-14 Created: 2022-12-14 Last updated: 2022-12-14Bibliographically approved

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Shiino, TakayukiGebresenbut, Girma HailuPay Gómez, CesarNordblad, PerMathieu, Roland

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Shiino, TakayukiGebresenbut, Girma HailuPay Gómez, CesarNordblad, PerMathieu, Roland
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