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Optical detection of valley-polarized electron diffusion in diamond
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Electrical Engineering, Electricity.ORCID iD: 0000-0001-7370-8171
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Electrical Engineering, Electricity.ORCID iD: 0000-0002-6057-7931
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Electrical Engineering, Electricity.ORCID iD: 0000-0002-8815-5992
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Electrical Engineering, Electricity.ORCID iD: 0000-0003-2197-5352
2023 (English)In: Materials for Quantum Technology, E-ISSN 2633-4356, Vol. 3, article id 025001Article in journal (Refereed) Published
Abstract [en]

Using the state of valley-polarization of electrons in solids is a promising new paradigm for information storage and processing. The central challenge in utilizing valley-polarization for this purpose is to develop methods for manipulating and reading out the final valley state. Here, we demonstrate optical detection of valley-polarized electrons in diamond. It is achieved by capturing images of electroluminescence from nitrogen-vacancy centers at the surface of a diamond sample that are excited by electrons drifting and diffusing through the sample. Monte Carlo simulations are performed to interpret the resulting experimental diffusion patterns. Our results give insight into the drift-diffusion of valley-polarized electrons in diamond and yield a way of analyzing the valley-polarization of ensembles of electrons.

Place, publisher, year, edition, pages
Institute of Physics Publishing (IOPP), 2023. Vol. 3, article id 025001
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-500803DOI: 10.1088/2633-4356/accac7ISI: 001146243700001Scopus ID: 2-s2.0-85153570509OAI: oai:DiVA.org:uu-500803DiVA, id: diva2:1752993
Funder
Magnus Bergvall Foundation, 2020-03615Helge Ax:son Johnsons stiftelse , F20-0342Swedish Research Council, 2018-04154Available from: 2023-04-25 Created: 2023-04-25 Last updated: 2025-02-18Bibliographically approved
In thesis
1. Low Temperature Charge Transport in Diamond
Open this publication in new window or tab >>Low Temperature Charge Transport in Diamond
2023 (English)Doctoral thesis, comprehensive summary (Other academic)
Abstract [en]

Diamond is a wide band semiconductor with fascinating electrical and physical properties. It has high thermal and electrical conductivity, high electrical breakdown field, high radiation hardness and is chemically inert. These properties make diamond an excellent material for high power electronics, high frequency electronics, particle detectors and for electronics in hazardous environments. Moreover, diamond has been suggested for applications in valleytronics.

Valleytronics is a term for semiconductor technology that exploits minima in an energy band, so called valleys. In diamond there are six of these valleys in the conduction band and the conduction electrons resides in one of these six valleys at low temperatures. The valley an electron is in, its valley polarization, affects how it behaves in an electric field. The valley polarization along with an understanding of the electron-phonon scattering processes makes a good framework for understanding of electron transport in diamond. In this thesis, both of these topics have been explored, with the purpose of understanding low temperature electron transport in diamond. A detailed description of low temperature charge transport is relevant for several reasons. Firstly, it can help with understanding the charge transport in e.g. detectors. Secondly, it gives more degrees of freedom when designing new electronics.   

In this thesis, both experiments and simulations has been used investigate low temperature transport in diamond. The main experiment method used was time-of-flight were the drift current of valley polarized electrons measured between two contacts. These experiment could then be compared with Monte Carlo simulations. The simulations gave valuable insigne into the dynamics of the electrons. This self-written code for Monte Carlo simulations is described in greater detail in this thesis. 

Some highlighted results of this thesis are as follows: optical observations of valley polarized diffusion, electrical control of valley polarized currents and the estimations of the acoustic deformation potentials to Du = 18.5 eV and Dd = -5.7 eV. This thesis also includes a more general part about charge transport.

Place, publisher, year, edition, pages
Uppsala: Acta Universitatis Upsaliensis, 2023. p. 100
Series
Digital Comprehensive Summaries of Uppsala Dissertations from the Faculty of Science and Technology, ISSN 1651-6214 ; 2273
National Category
Other Electrical Engineering, Electronic Engineering, Information Engineering
Research subject
Engineering Science with specialization in Electronics
Identifiers
urn:nbn:se:uu:diva-500810 (URN)978-91-513-1820-2 (ISBN)
Public defence
2023-06-08, Polhemsalen, Lägerhyddsvägen 1, Uppsala, 09:15 (English)
Opponent
Supervisors
Available from: 2023-05-15 Created: 2023-04-25 Last updated: 2024-01-18

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Djurberg, ViktorMajdi, SamanSuntornwipat, NattakarnIsberg, Jan

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