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2D Layered Nanomaterials as Fillers in Polymer Composite Electrolytes for Lithium Batteries
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström.
Ulm Univ, Inst Inorgan Chem 1, Albert Einstein Allee 11, D-89081 Ulm, Germany..
CSIR, Natl Chem Lab NCL, Dr Homi Bhabha Rd, Pune 411008, India..
CSIR, Natl Chem Lab NCL, Dr Homi Bhabha Rd, Pune 411008, India..
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2023 (English)In: Advanced Energy Materials, ISSN 1614-6832, E-ISSN 1614-6840, Vol. 13, no 15, article id 2203326Article, review/survey (Refereed) Published
Abstract [en]

Polymer composite electrolytes (PCEs), i.e., materials combining the disciplines of polymer chemistry, inorganic chemistry, and electrochemistry, have received tremendous attention within academia and industry for lithium-based battery applications. While PCEs often comprise 3D micro- or nanoparticles, this review thoroughly summarizes the prospects of 2D layered inorganic, organic, and hybrid nanomaterials as active (ion conductive) or passive (nonion conductive) fillers in PCEs. The synthetic inorganic nanofillers covered here include graphene oxide, boron nitride, transition metal chalcogenides, phosphorene, and MXenes. Furthermore, the use of naturally occurring 2D layered clay minerals, such as layered double hydroxides and silicates, in PCEs is also thoroughly detailed considering their impact on battery cell performance. Despite the dominance of 2D layered inorganic materials, their organic and hybrid counterparts, such as 2D covalent organic frameworks and 2D metal-organic frameworks are also identified as tuneable nanofillers for use in PCE. Hence, this review gives an overview of the plethora of options available for the selective development of both the 2D layered nanofillers and resulting PCEs, which can revolutionize the field of polymer-based solid-state electrolytes and their implementation in lithium and post-lithium batteries.

Place, publisher, year, edition, pages
Wiley-VCH Verlagsgesellschaft, 2023. Vol. 13, no 15, article id 2203326
Keywords [en]
2D materials, clay minerals, covalent organic frameworks, metal-organic frameworks, MXene, polymer composite electrolyte, solid-state batteries
National Category
Materials Chemistry Inorganic Chemistry
Identifiers
URN: urn:nbn:se:uu:diva-513060DOI: 10.1002/aenm.202203326ISI: 000947031300001OAI: oai:DiVA.org:uu-513060DiVA, id: diva2:1805257
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EU, European Research CouncilStandUpAvailable from: 2023-10-16 Created: 2023-10-16 Last updated: 2023-10-16Bibliographically approved

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Mindemark, JonasBrandell, Daniel

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