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Real-time observation of non-equilibrium phonon-electron energy and angular momentum flow in laser-heated nickel
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, FREIA.ORCID iD: 0000-0001-7257-7309
DESY, D-22607 Hamburg, Germany..
DESY, D-22607 Hamburg, Germany..
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, FREIA.ORCID iD: 0000-0003-3667-8334
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2024 (English)In: Science Advances, E-ISSN 2375-2548, Vol. 10, no 5, article id eadj2407Article in journal (Refereed) Published
Abstract [en]

Identifying the microscopic nature of non-equilibrium energy transfer mechanisms among electronic, spin, and lattice degrees of freedom is central to understanding ultrafast phenomena such as manipulating magnetism on the femtosecond timescale. Here, we use time- and angle-resolved photoemission spectroscopy to go beyond the often-used ensemble-averaged view of non-equilibrium dynamics in terms of quasiparticle temperature evolutions. We show for ferromagnetic Ni that the non-equilibrium electron and spin dynamics display pronounced variations with electron momentum, whereas the magnetic exchange interaction remains isotropic. This highlights the influence of lattice-mediated scattering processes and opens a pathway toward unraveling the still elusive microscopic mechanism of spin-lattice angular momentum transfer.

Place, publisher, year, edition, pages
American Association For Cancer Research (AACR), 2024. Vol. 10, no 5, article id eadj2407
National Category
Condensed Matter Physics Atom and Molecular Physics and Optics
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URN: urn:nbn:se:uu:diva-526897DOI: 10.1126/sciadv.adj2407ISI: 001185617600008PubMedID: 38295169OAI: oai:DiVA.org:uu-526897DiVA, id: diva2:1852952
Funder
Swedish Research CouncilCarl Tryggers foundation Swedish Research CouncilKnut and Alice Wallenberg Foundation, 2022.0079German Research Foundation (DFG), 328545488Available from: 2024-04-19 Created: 2024-04-19 Last updated: 2024-04-19Bibliographically approved

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Shokeen, VishalWang, XiaocuiYaroslavtsev, AlexanderMaldonado, PabloBerritta, MarcoOppeneer, Peter M.Dürr, Hermann

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Shokeen, VishalWang, XiaocuiYaroslavtsev, AlexanderMaldonado, PabloBerritta, MarcoWenthaus, LukasOppeneer, Peter M.Schönhense, GerdDürr, Hermann
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