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Electrochemical Seawater Oxidation by (Ni,Co)3O4-RuO2 Catalysts at Neutral pH in a Forward Osmosis Cell
Stockholm Univ, Dept Mat & Environm Chem, SE-10691 Stockholm, Sweden..
Stockholm Univ, Dept Mat & Environm Chem, SE-10691 Stockholm, Sweden..
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Materials Science and Engineering, Solid State Physics.
Uppsala University, Disciplinary Domain of Science and Technology, Technology, Department of Materials Science and Engineering, Solid State Physics.ORCID iD: 0000-0002-0671-435X
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2024 (English)In: ACS Applied Energy Materials, E-ISSN 2574-0962, Vol. 7, no 10, p. 4445-4453Article in journal (Refereed) Published
Abstract [en]

Using seawater to generate green hydrogen through electrolysis is a promising strategy for energy conversion. However, direct seawater splitting to form green hydrogen suffers drawbacks from electrode corrosion due to chlorine and other impurities. Herein, we demonstrate direct electrochemical seawater splitting using a forward osmosis membrane coupled with an electrolysis cell. By using this cell, high activity (270 mV at 10 mA/cm2) and decent stability (up to 6 days) are achieved by utilizing RuO2-(Ni,Co)3O4 catalyst in a neutral electrolyte. This system is further studied in various electrolytes under neutral to alkaline conditions. This proof of concept shows that seawater splitting could be coupled with semipermeable membranes, allowing for direct utilization of seawater without pretreatment or purification and evading the challenges posed by impurities.

Place, publisher, year, edition, pages
American Chemical Society (ACS), 2024. Vol. 7, no 10, p. 4445-4453
Keywords [en]
seawater, electrolysis, forwardosmosis, oxygen evolution, water splitting
National Category
Energy Engineering Other Chemistry Topics
Identifiers
URN: urn:nbn:se:uu:diva-541411DOI: 10.1021/acsaem.4c00386ISI: 001225280300001OAI: oai:DiVA.org:uu-541411DiVA, id: diva2:1909578
Funder
Knut and Alice Wallenberg Foundation, KAW 2003.0198Swedish Foundation for Strategic Research, EM16-0010Swedish Research Council, 2019-00207Olle Engkvists stiftelse, 211-0067Available from: 2024-10-31 Created: 2024-10-31 Last updated: 2024-10-31Bibliographically approved

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Anil, AthiraSalazar-Alvarez, Germán

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