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Modeling Pu-239 Fission Fragment De-Excitation applying the Total Monte Carlo method in TALYS
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy.
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Applied Nuclear Physics.ORCID iD: 0000-0002-1233-0221
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Applied Nuclear Physics.ORCID iD: 0000-0002-4442-2569
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Applied Nuclear Physics.ORCID iD: 0009-0003-4014-7605
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2025 (English)In: 7TH INTERNATIONAL WORKSHOP ON COMPOUND-NUCLEAR REACTIONS AND RELATED TOPICS, CNR*24 / [ed] Dimitriou, P Capote, R Schnabel, G, EDP Sciences, 2025, Vol. 322, article id 07005Conference paper, Published paper (Refereed)
Abstract [en]

In this study, we applied the Total Monte Carlo (TMC) methodology in de-excitation simulations of primary fission fragments (FF) using the TALYS code. The goal was to develop and optimise a methodology to benchmark initial fission model assumptions on fission mass yield distributions, excitation energy sharing and angular momentum population. The study was performed on the thermal neutron induced fission of Pu-239(n(th),f). The work aimed at evaluating fission model deficiencies and parameter sensitivities. We systematically varied TALYS input data by generating 5000 random files through the GEF code, randomizing 94 model parameters that affect fission yields and energy distributions within 3% of their default values. This variation revealed significant changes in the fission observables, such as prompt neutron and gamma-ray multiplicities and energy spectra. The results indicate some systematic defects in the assumed excitation-energies and angular momenta. Another outcome from the study is the identification of a need for new correlation measurements on prompt neutrons and gamma-rays from the Pu-239(n(th),f) reaction, as well as an updated evaluation.

Place, publisher, year, edition, pages
EDP Sciences, 2025. Vol. 322, article id 07005
Series
EPJ Web of Conferences, ISSN 2100-014X
National Category
Subatomic Physics
Identifiers
URN: urn:nbn:se:uu:diva-556713DOI: 10.1051/epjconf/202532207005ISI: 001453120000032Scopus ID: 2-s2.0-105002340927OAI: oai:DiVA.org:uu-556713DiVA, id: diva2:1959327
Conference
7th International Workshop on Compound-Nuclear Reactions and Related Topics-CNR, JUL 08-12, 2024, Vienna, AUSTRIA
Funder
Swedish Research Council, 2019-05385Swedish Energy Agency, P2023-01281Available from: 2025-05-20 Created: 2025-05-20 Last updated: 2025-05-20Bibliographically approved

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Karlsson, PeterAl-Adili, AliGöök, AlfGao, ZhihaoPomp, StephanSjöstrand, HenrikSolders, Andreas

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