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Chiral spin and orbital angular momentum textures in Mn chains on W(110): Interplay of spin-orbit coupling and crystal-field effects
Univ Fed Oeste Para, Inst Engn & Geociencias, Santarem, PA, Brazil..
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory.ORCID iD: 0000-0002-4238-5733
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory.ORCID iD: 0000-0002-5134-1978
Univ Fed Fluminense, Inst Fis, BR-24210346 Niteroi, RJ, Brazil..
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2025 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 112, no 1, article id 014440Article in journal (Refereed) Published
Abstract [en]

Stabilization of unusual spin-orbit-driven magnetic orderings are achieved for chains of Mn atoms deposited on a W(110) substrate. First-principles electronic structure calculations show that the ground-state spin configuration is noncollinear, forming chiral spiral-like structures, driven by competing nearest-and next-nearest-neighbor interactions. The orbital magnetic moments are also found to exhibit noncollinear ordering that, interestingly, tend to align in-plane for some systems with an orientation distinctly differently from that of the spin moment. We analyze the mechanism behind such behavior, and find that it is due to the competition between the spin-orbit interaction and crystal-field splitting. Model calculations based on this assumption reproduce the main findings observed in our first-principles calculations.

Place, publisher, year, edition, pages
American Physical Society, 2025. Vol. 112, no 1, article id 014440
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-565051DOI: 10.1103/s6b9-djksISI: 001538319000003OAI: oai:DiVA.org:uu-565051DiVA, id: diva2:1990127
Part of project
2D magnets for spintronic and magnonic applications, Swedish Research Council
Funder
EU, European Research Council, 854843Knut and Alice Wallenberg FoundationSwedish Research Council, 2019-03569Available from: 2025-08-19 Created: 2025-08-19 Last updated: 2025-08-19Bibliographically approved

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Kvashnin, Yaroslav O.Bergman, AndersEriksson, OlleKatsnelson, Mikhail I.

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Materials Theory
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Physical Review B
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