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Element-Selective Probing of Ultrafast Ferromagnetic-Antiferromagnetic Order Dynamics in Fe/CoO Bilayers
Free Univ Berlin, Inst Expt Phys, Arnimallee 14, D-14195 Berlin, Germany..
Free Univ Berlin, Inst Expt Phys, Arnimallee 14, D-14195 Berlin, Germany..
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory. Free Univ Berlin, Inst Expt Phys, Arnimallee 14, D-14195 Berlin, Germany.ORCID iD: 0000-0002-3283-2560
Free Univ Berlin, Inst Expt Phys, Arnimallee 14, D-14195 Berlin, Germany..
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2026 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 136, no 12, article id 126705Article in journal (Refereed) Published
Abstract [en]

The ultrafast magnetization dynamics of an epitaxial Fe/CoObilayer on Ag(001) is examined in an element-resolved way by resonant soft-x-ray reflectivity. The transient magnetic linear dichroism at the Co 𝐿2 edge and the magnetic circular dichroism at the Fe 𝐿3 edge measured in reflection in a pump–probe experiment with 120 fs temporal resolution show the loss of antiferromagnetic and ferromagnetic order in CoO and Fe, respectively, both within 300 fs after excitation with 60 fs light pulses of 800 and 400 nm wavelengths. A comparison to spin-dynamics simulations using an atomistic spin model shows that direct energy transfer from the laser-excited electrons in Fe to the magnetic moments in CoO provides the dominant demagnetization channel in the case of 800-nm excitation.

Place, publisher, year, edition, pages
American Physical Society, 2026. Vol. 136, no 12, article id 126705
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Condensed Matter Physics
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URN: urn:nbn:se:uu:diva-585483DOI: 10.1103/gcwk-tsj5ISI: 001746124100003PubMedID: 41965035Scopus ID: 2-s2.0-105034591860OAI: oai:DiVA.org:uu-585483DiVA, id: diva2:2058240
Funder
Swedish Research Council, 2022-06725Available from: 2026-05-07 Created: 2026-05-07 Last updated: 2026-05-07Bibliographically approved

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Weißenhofer, MarkusOppeneer, Peter M.

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